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Type of Document	Dissertation
Author	Maier, Stefan Alexander
Author's Email Address	stmaier AT caltech.edu
URN	etd-02062003-155401
Persistent URL	http://resolver.caltech.edu/CaltechETD:etd-02062003-155401
Title	Guiding of electromagnetic energy in subwavelength periodic metal structures
Degree	PhD
Option	Applied Physics
Advisory Committee	Advisor Name Title Harry Atwater Committee Chair Julia Kornfield Committee Member Kerry Vahala Committee Member Oskar Painter Committee Member Stephen Quake Committee Member
Keywords	near-field optics metal nanoparticles nano-optics nano-waveguides plasmon-polariton plasmon waveguides
Date of Defense	2003-01-24
Availability	unrestricted
Abstract The ultimate miniaturization of optical devices requires structures that guide electromagnetic energy with a lateral confinement below the diffraction limit of light. In this thesis, the possibility of employing plasmon-polariton excitations in plasmon waveguides consisting of closely spaced metal nanoclusters for this purpose is examined. The feasibility of energy transport with mode sizes below the diffraction limit of visible light over distances of several hundred nanometers is demonstrated. As a macroscopic analogue to plasmon waveguides, the transport of electromagnetic energy in the microwave regime along closely spaced centimeter-scale metal rods is examined. Full-field electrodynamic simulations show that information transport occurs at a group velocity of 0.65c for fabricated structures consisting of copper rods excited at 8 GHz. A variety of passive routing structures and an all-optical modulator are demonstrated. The possibility of guiding electromagnetic energy at visible frequencies with mode sizes below the diffraction limit using plasmon waveguides is analyzed using a point-dipole model and finite-difference time-domain simulations. It is shown that energy transport occurs via near-field coupling between metal nanoparticles, which leads to coherent propagation of energy. For spherical gold particles in air, group velocities up to 0.06c are demonstrated, and a change in particle shape to spheroidal particles shows up to a threefold increase in group velocity. Pulses with transverse polarization are shown to propagate with negative phase velocities antiparallel to the energy flow. Plasmon waveguides consisting of gold and silver nanoparticles were fabricated using electron beam lithography. The key parameters that govern the energy transport are determined for various interparticle spacings and particle chain lengths using far-field measurements of the collective plasmon modes. Spherical gold nanoparticles with a diameter of 50 nm and an interparticle spacing of 75 nm show an energy attenuation of 6 dB/30 nm. This loss can be reduced by one order of magnitude by a geometry change to spheroidal particles. Using the tip of a near-field optical microscope as a local excitation source and fluorescent nanospheres as detectors, experimental evidence for energy transport over a distance of 0.5 micron is presented for plasmon waveguides consisting of silver rods with a 3:1 aspect ratio.
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